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Chemical Engineering of Fused MetalloPorphyrins Thin Films for the Clean Production of Hydrogen

Project description

Clean hydrogen production enabled by metalloporphyrins

The current worldwide energy and environmental crisis creates an urgent need for new solutions. The EU-funded CLEANH2 project will help engineer these new solutions by developing a new class of materials for the clean and efficient production of hydrogen from ‘solar water splitting’ (generating molecular hydrogen and oxygen for fuel cells). The project concept relies on the gas phase reaction of metalloporphyrins –attractive molecules for water splitting – to engineer new heterogeneous catalysts with remarkable hydrogen production yields. The field is still relatively unexplored but if this breakthrough proves successful, it could support a new economy built on hydrogen instead of fossil fuels.

Objective

This project stands in the general context of the current worldwide energy and environmental crisis. It aims to engineer a new generation of conjugated microporous polymers based on fused metalloporphyrins for the low-cost, clean and efficient production of hydrogen from solar water splitting. The CLEANH2 concept relies on the gas phase reaction of metalloporphyrins to engineer new heterogeneous catalysts with remarkable hydrogen production yields. Metalloporphyrins, selected by Nature to fulfil the main catalytic phenomena allowing life, are attractive molecules for water splitting owing to their highly conjugated structure and central metal ion, which can readily interconvert between different oxidation states to accomplish oxidation and reduction reactions. For efficiency and sustainability considerations, it is highly desirable to employ metalloporphyrins in conductive assemblies for heterogeneous catalysis. Nevertheless, due to the lack of synthetic approach, the design and application of conjugated porphyrin assemblies is a largely unexplored topic in view of the plethora of available porphyrin patterns.
The central idea of CLEANH2 builds upon our recent advance in the gas phase synthesis and deposition of directly fused metalloporphyrins coatings. Progress in our approach is expected to open the way for the construction of powerful catalytic and photocatalytic materials. To achieve this, the key challenging goals of this project are: 1) the engineering of the microstructure and electronic structure of directly fused metalloporphyrins thin films; 2) the use of the full potential of directly fused metalloporphyrins thin films for the unmet, clean and high quantum yield overall water splitting for hydrogen production. The outcomes of CLEANH2 will be foundational for the engineering of directly fused metalloporphyrins systems and their implementation in advanced technological applications related to catalysis and solar energy.

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Keywords

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Programme(s)

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Topic(s)

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Funding Scheme

Funding scheme (or “Type of Action”) inside a programme with common features. It specifies: the scope of what is funded; the reimbursement rate; specific evaluation criteria to qualify for funding; and the use of simplified forms of costs like lump sums.

ERC-COG - Consolidator Grant

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Call for proposal

Procedure for inviting applicants to submit project proposals, with the aim of receiving EU funding.

(opens in new window) ERC-2019-COG

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Host institution

LUXEMBOURG INSTITUTE OF SCIENCE AND TECHNOLOGY
Net EU contribution

Net EU financial contribution. The sum of money that the participant receives, deducted by the EU contribution to its linked third party. It considers the distribution of the EU financial contribution between direct beneficiaries of the project and other types of participants, like third-party participants.

€ 1 900 711,00
Address
5 AVENUE DES HAUTS FOURNEAUX
4362 Esch Sur Alzette
Luxembourg

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Region
Luxembourg Luxembourg Luxembourg
Activity type
Research Organisations
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Total cost

The total costs incurred by this organisation to participate in the project, including direct and indirect costs. This amount is a subset of the overall project budget.

€ 1 900 711,00

Beneficiaries (1)

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